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The GC Computer Code for Flow Sheet Simulation of Pyrochemical Processing of Spent Nuclear Fuels

Rajesh K. Ahluwalia, Howard K. Geyer

Nuclear Technology / Volume 116 / Number 2 / November 1996 / Pages 180-195

Technical Paper / Enrichment and Reprocessing System / dx.doi.org/10.13182/NT96-A35299

The GC computer code has been developed for flow sheet simulation of pyrochemical processing of spent nuclear fuel. It utilizes a robust algorithm SLG for analyzing simultaneous chemical reactions between species distributed across many phases. Models have been developed for analysis of the oxide fuel reduction process, salt recovery by electrochemical decomposition of lithium oxide, uranium separation from the reduced fuel by electrorefining, and extraction of fission products into liquid cadmium. The versatility of GC is demonstrated by applying the code to a flow sheet of current interest.