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Photon Activation Analysis in Gallium, Nickel, and Vanadium

Robert Bentley, Geno Santistevan, Douglas Wells, Andrew Hutton, Adam Stavola, Steve Benson, Kevin Jordan, Joe Gubeli, Pavel Degtiarenko, Lila Dabill

Nuclear Science and Engineering / Volume 198 / Number 1 / January 2024 / Pages 158-166

Research Article / dx.doi.org/10.1080/00295639.2023.2180265

Received:October 18, 2022
Accepted:February 10, 2023
Published:December 12, 2023

This research explored the development of the photonuclear production method of Cu from Ga as well as Sc from V. Both products serve as high-demand research medical radioisotopes. Furthermore, an understanding of these reactions is significant to fundamental nuclear physics and astrophysics. Bremsstrahlung flux was induced by an electron linac and a 1-mm tungsten radiator. Irradiation of gallium oxide powder, 98.78% pure Ga, and a natural vanadium foil at 30.9 MeV and 100 W for 1 h produced 64.4 ± 0.4 Bq/W·s·kg of Cu and 164 ± 3.1 Bq/W·s·kg of Sc. A secondary irradiation with 99.6% pure Ga and natural vanadium at 31.5 MeV and 100 W for 1.1 h produced 79.8 ± 0.9 Bq/W·s·kg of Cu and 136 ± 7.2 Bq/W·s·kg of Sc. The photoinduced activation is promising; however, further research into optimal geometry and power is required to maximize specific activity. Natural nickel was also irradiated to serve as a benchmark comparison. Effective cross sections for each reaction were inferred.